Paper No. 8
Presentation Time: 10:20 AM

THE RESPONSE OF A GROUNDWATER MICROBIAL COMMUNITY TO VARIATIONS IN THE BIOGEOCHEMISTRY OF RECHARGE WATERS: INSIGHTS FROM AN EOGENEIC CARBONATE AQUIFER


COOPER, Katherine J.1, WHITAKER, Fiona F.1, ANESIO, Alexandre M.2, NAISH, Miranda1 and REYNOLDS, Darren3, (1)University of Bristol, School of Earth Sciences, Wills Memorial Building, Queens Road, Bristol, BS8 1RJ, United Kingdom, (2)University of Bristol, School of Geographical Sciences, University Road, Bristol, BS8 1SS, United Kingdom, (3)University of the West of England, Applied Sciences, Frenchay Campus, Coldharbour Lane, Bristol, BS16 1QY, United Kingdom, k.j.cooper@bristol.ac.uk

Most freshwater recharge in tropical karstic aquifers occurs during intense rainfall events. The composition of waters that reach the water table is strongly influenced by interaction of the rainfall with vegetation, soil, epikarst and/or the unsaturated zone. Along complex and varied pathways, fresh dissolved organic carbon may be incorporated within recharge waters, and subsurface oxidation of this organic carbon may drive carbonate dissolution at and below the water table.

This study investigates the response of the natural microbial community within a shallow eogenetic carbonate aquifer on North Andros Island, Bahamas, to inputs of differing concentrations and compositions of dissolved organic carbon (DOC) sourced from various recharge pathways. During an individual storm, geochemical modification of rainfall was evaluated within throughflow, stemflow, overland flow and infiltration through the epikarst. The total concentration of DOC was measured and its composition was characterised using fluorescence spectroscopy. The biological oxygen demand (BOD) of subsamples of the shallow groundwater inoculated with different recharge waters was measured to determine the bioavailability fraction of the DOC.

There were distinct geochemical differences between the types of recharge waters, driven mostly by interaction with organic acids, with stemflow having a very low pH when compared to the rainfall. The majority of recharge waters stimulated significant microbial respiration relative to the control, with this response differing between the samples. However, the BOD does not correlate directly with the total concentration of DOC in the samples. Fluorescence spectroscopy highlighted differences between the characteristics of the DOC, with the degree of interaction with vegetation being a dominant factor controlling the composition. There was a strong positive correlation between the ratio of C:A peaks, the two peaks relating to humic-like substances, and the BOD. The C peak has previously been noted to represent microbially reworked aromatic and aliphatic fulvic-like substance. This suggests that a by-product of the respiration of the microbial community at the shallow water table could be an increase in C peak abundance, which could be used as a proxy for microbial response within the aquifer.