Joint 56th Annual North-Central/ 71st Annual Southeastern Section Meeting - 2022

Paper No. 26-5
Presentation Time: 9:05 AM

GEOLOGIC CONTROLS ON 137CS CYCLING BY TERRESTRIAL VEGETATION IN THE EASTERN U.S


CHELLMAN, Kathleen O'Hara and KASTE, J.M., Department of Geology, College of William & Mary, Williamsburg, VA 23187

137Cs is a radioactive trace metal (T1/2 = 30 y) which was dispersed globally by nuclear weapons testing in the 1950s-1960s. Prevailing winds caused some areas far from the test sites to receive significant fallout, which is still easily measured in soils, sediments and even some vegetation in the Eastern United States. Recent work near Chernobyl and Fukushima indicates that trace levels of 137Cs can harm insects and ecological function. It’s been established that in areas with low soil potassium, 137Cs is cycled in vegetation; however, soil potassium alone doesn't consistently predict the 137Cs content of plants. We hypothesize that local geology more broadly influences the cycling of 137Cs by vegetation, which ultimately controls potassium concentrations, clay mineralogy, and slope. We collected foliage and soil samples from sites in Tennessee and Virginia to examine geologic controls affecting 137Cs uptake in vegetation. Our sites span Conglomerate, Quartzite, Dolostone, Graywacke, and detrital sediment. Across this gradient of soil parent material, foliage concentrations of 137Cs ranged from undetected (0.1 Bq/kg) to 5.7 Bq/kg. Foliage at each site had widely varying 137Cs, indicating that there is a species control on uptake. By comparing the ratio of 137Cs in plants to soil, I found Quartzite bedrock showed almost no 137Cs uptake, and Graywacke had the highest with a median of 21%. The next steps are to examine plant available potassium and illite content in the soil samples from each site. This research will help us understand how geology affects 137Cs and trace metal cycling and thus predict which plant or animal species could be at increased risk to radiation exposure.